We present a combined experimental and numerical study of the far-field emission properties of optical travelling wave antennas made from low-loss dielectric materials. The antennas considered here are composed of two simple building blocks, a director and a reflector, deposited on a glass substrate. Colloidal quantum dots placed in the feed gap between the two elements serve as internal light source. The emission profile of the antenna is mainly formed by the director while the reflector suppresses backward emission. Systematic studies of the director dimensions as well as variation of antenna material show that the effective refractive index of the director primarily governs the far-field emission pattern. Below cut off, i.e., if the director’s effective refractive index is smaller than the refractive index of the substrate, the main lobe results from leaky wave emission along the director. In contrast, if the director supports a guided mode, the emission predominately originates from the end facet of the director.

Employing the ultrafast control of electronic states of a semiconductor quantum dot in a cavity, we introduce an approach to achieve on-demand emission of single photons with almost perfect indistinguishability and photon pairs with near ideal entanglement. Our scheme is based on optical excitation off resonant to a cavity mode followed by ultrafast control of the electronic states using the time-dependent quantum-confined Stark effect, which then allows for cavity-resonant emission. Our theoretical analysis considers cavity-loss mechanisms, the Stark effect, and phonon-induced dephasing, allowing realistic predictions for finite temperatures.

We demonstrate the integration of amorphous tungsten silicide superconducting nanowire single-photon detectors on titanium in-diffused lithium niobate waveguides. We show proof-of-principle detection of evanescently coupled photons of 1550 nm wavelength using bidirectional waveguide coupling for two orthogonal polarization directions. We investigate the internal detection efficiency as well as detector absorption using coupling-independent characterization measurements. Furthermore, we describe strategies to improve the yield and efficiency of these devices.

Gaussian-beam-like bundles of semi-guided waves propagating in a dielectric slab can excite modes with high-order optical angular momentum supported by a circular fiber. We consider a multimode step-index fiber with a high-index coating, where the waves in the slab are evanescently coupled to the modes of the fiber. Conditions for effective resonant interaction are identified. Based on a hybrid analytical–numerical coupled mode model, our simulations predict that substantial fractions of the input power can be focused into waves with specific orbital angular momentum, of excellent purity, with a clear distinction between degenerate modes with opposite vorticity.

A dielectric step-index optical fiber with tube-like profile is considered, being positioned with a small gap on top of a dielectric slab waveguide. We propose a 2.5-D hybrid analytical/numerical coupled mode model for the evanescent excitation of the tube through semi-guided waves propagating in the slab at oblique angles. The model combines the directional polarized modes supported by the slab with analytic solutions for the TE-, TM-, and orbital-angular-momentum (OAM) modes of the tube-shaped fiber. Implementational details of the scheme are discussed, complemented by finite-element simulations for verification purposes. Our results include configurations with resonant in-fiber excitation of OAM modes with large orbital angular momentum and strong field enhancement.

We numerically simulate multiple light scattering in discrete disordered media represented by large clusters of irregular non-absorbing particles. The packing density of clusters is 0.5. With such conditions diffuse scattering is significantly reduced and light transport follows propagation channels that are determined by the particle size and topology of the medium. This kind of localization produces coherent backscattering intensity surge and enhanced negative polarization branch if compared to lower density samples.

The challenge of designing new tunable nonlinear dielectric materials with tailored properties has attracted an increasing amount of interest recently. Herein, we study the effective nonlinear dielectric response of a stochastic paraelectric-dielectric composite consisting of equilibrium distributions of circular and partially penetrable disks (or parallel, infinitely long, identical, partially penetrable, circular cylinders) of a dielectric phase randomly dispersed in a continuous matrix of a paraelectric phase. The random microstructures were generated using the Metropolis Monte Carlo algorithm. The evaluation of the effective permittivity and tunability were carried out by employing either a Landau thermodynamic model or its Johnson’s approximation to describe the field-dependent permittivity of the paraelectric phase and solving continuum-electrostatics equations using finite element calculations. We reveal that the percolation threshold in this composite governs the critical behavior of the effective permittivity and tunability. For microstructures below the percolation threshold, our simulations demonstrate a strong nonlinear behaviour of the field-dependent effective permittivity and very high tunability that increases as a function of dielectric phase concentration. Above the percolation threshold, the effective permittivity shows the tendency to linearization and the tunability dramatically drops down. The highly reduced permittivity and extraordinarily high tunability are obtained for the composites with dielectric impenetrable disks at high concentrations, in which the triggering of the percolation transition is avoided. The reported results cast light on distinct nonlinear behaviour of 2D and 3D stochastic composites and can guide the design of novel composites with the controlled morphology and tailored permittivity and tunability.

A stepwise angular spectrum method (SASM) for curved interfaces is presented to calculate the wave propagation in planar lens-like integrated optical structures based on photonic slab waveguides. The method is derived and illustrated for an effective 2D setup first and then for 3D slab waveguide lenses. We employ slab waveguides of different thicknesses connected by curved surfaces to realize a lens-like structure. To simulate the wave propagation in 3D including reflection and scattering losses, the stepwise angular spectrum method is combined with full vectorial finite element computations for subproblems with lower complexity. Our SASM results show excellent agreement with rigorous numerical simulations of the full structures with a substantially lower computational effort and can be utilized for the simulation-based design and optimization of complex and large scale setups.

We consider light scattering from a new type of model particle whose shape is represented in the form of a generalized ellipsoid having N foci, where N is greater than two. Such particles can be convex as well as concave. We use the geometrical optics approximation to study the light scattering from 3-foci particles. Non-zero elements of the scattering matrix are calculated for ensembles of randomly oriented independent transparent particles, m = n + i0. Several internal reflection orders are considered separately. It was found that the transmission-transmission (TT) and transmission-reflectance-transmission (TRT) components dominate in the formation of intensity of scattered light at large and small phase angles, respectively. We found a significant role of the total internal reflections of the TRT in the middle portion of the phase angle range. The main factors in the formation of positive linear polarization are the R and TRT component. The TT component is responsible for the formation of negative polarization branch at large phase angles.

A rectangular dielectric strip at some distance above an optical slab waveguide is being considered, for evanescent excitation of the strip through the semi-guided waves supported by the slab, at specific oblique angles. The 2.5-D configuration shows resonant transmission properties with respect to variations of the angle of incidence, or of the excitation frequency, respectively. The strength of the interaction can be controlled by the gap between strip and slab. For increasing distance, our simulations predict resonant states with unit extremal reflectance of an angular or spectral width that tends to zero, i.e. resonances with a Q-factor that tends to infinity, while the resonance position approaches the level of the guided mode of the strip. This exceptionally simple system realizes what might be termed a “bound state coupled to the continuum”.

We investigate optical microresonators consisting of either one or two coupled rectangular strips between upper and lower slab waveguides. The cavities are evanescently excited under oblique angles by thin-film guided, in-plane unguided waves supported by one of the slab waveguides. Beyond a specific incidence angle, losses are fully suppressed. The interaction between the guided mode of the cavity-strip and the incoming slab modes leads to resonant behavior for specific incidence angles and gaps. For a single cavity, at resonance, the input power is equally split among each of the four output ports, while for two cavities an add-drop filter can be realized that, at resonance, routes the incoming power completely to the forward drop waveguide via the cavity. For both applications, the strength of the interaction is controlled by the gaps between cavities and waveguides.

We report on the coherent phase manipulation of quantum dot excitons by electric means. For our experiments, we use a low capacitance single quantum dot photodiode which is electrically controlled by a custom designed SiGe:C BiCMOS chip. The phase manipulation is performed and quantified in a Ramsey experiment, where ultrafast transient detuning of the exciton energy is performed synchronous to double pulse p/2 ps laser excitation. We are able to demonstrate electrically controlled phase manipulations with magnitudes up to 3p within 100 ps which is below the dephasing time of the quantum dot exciton.

Polarization of light is essential for some living organisms and many optical applications. Here, an orientation dependent polarization conversion effect is reported for light reflected from diamond‐structure‐based photonic crystals (D‐structure) inside the scales of a beetle, the weevil Entimus imperialis. When linearly polarized light propagates along its 〈100〉 directions, the D‐structure behaves analogous to a half‐wave plate in reflection but based on a different mechanism. The D‐structure rotates the polarization direction of linearly polarized light, and reflects circularly polarized light of both handednesses without changing it. This polarization effect is different from circular dichroism occurring in chiral biological photonic structures discovered before. The structural origin of this effect is symmetry breaking inside D‐structure's unit cell. This finding demonstrates that natural photonic structures can exploit multiple functionalities inherent to the design principles of their structural organization. Aiming at transferring the inherent polarization effect of the biological D‐structure to technically realizable materials, three simplified biomimetic structural models are derived and it is theoretically demonstrated that they retain the effect. Out of these structures, functioning woodpile structure prototypes are fabricated.

Metal nanoparticles host localized plasmon excitations that allow the manipulation of optical fields at the nanoscale. Despite the availability of several techniques for imaging plasmons, direct access into the symmetries of these excitations remains elusive, thus hindering progress in the development of applications. Here, we present a combination of angle-, polarization-, and space-resolved cathodoluminescence spectroscopy methods to selectively access the symmetry and degeneracy of plasmonic states in lithographically fabricated gold nanoprisms. We experimentally reveal and spatially map degenerate states of multipole plasmon modes with nanometer spatial resolution and further provide recipes for resolving optically dark and out-of-plane modes. Full-wave simulations in conjunction with a simple tight-binding model explain the complex plasmon structure in these particles and reveal intriguing mode-symmetry phenomena. Our approach introduces systematics for a comprehensive symmetry characterization of plasmonic states in high-symmetry nanostructures.

We study the dependence of the intensity and linear polarization of light scattered by isolated particles with the compact irregular shape on their size using the discontinuous Galerkin time domain numerical method. The size parameter of particles varies in the range of X = 10 to 150, and the complex refractive index is m = 1.5 + 0i. Our results show that the backscattering negative polarization branch weakens monotonously, but does not disappear at large sizes, up to the geometrical optics regime, and can be simulated without accounting for wave effects. The intensity backscattering surge becomes narrower with increasing particle size. For X = 150, the surge width is several degrees.

Oblique propagation of semi-guided waves across slab waveguide structures with bent corners is investigated. A critical angle can be defined beyond which all radiation losses are suppressed. Additionally an increase of the curvature radius of the bends also leads to low-loss configurations for incidence angles below that critical angle. A combination of two bent corner systems represents a step-like structure, behaving like a Fabry-Perot interferometer, with two partial reflectors separated by the vertical height between the horizontal slabs. We numerically analyse typical high-index-contrast Si/SiO2 structures for their reflectance and transmittance properties. When increasing the curvature radius the resonant effect becomes less relevant such that full transmittance is reached with less critical conditions on the vertical distance or the incidence angle. For practical interest 3-D problems are considered, where the structures are excited by the fundamental mode of a wide, shallow rib waveguide. High transmittance levels can be observed also for these 3-D configurations depending on the width of the rib.

We numerically simulate the circular polarization ratio of the radar signal backscattered from a large-grain cometary coma and compare the simulation results with the radar measurements for seven comets. We apply the discrete dipole approximation method and a model of random irregular particles. Our results confirm water ice composition of the cm-sized chunks detected by the NASA Deep Impact space probe in the vicinity of the nucleus of Comet 103P/Hartley 2. The index of the power-law size distribution in this case can be constrained to the range n ≈ 3.3–4.3. For the other considered comets the circular polarization ratio can be reproduced with variations of the power index between 2 and 5.

The 3D implementation of a hybrid analytical/numerical variant of the coupled-mode theory is discussed. Eigenmodes of the constituting dielectric channels are computed numerically. The frequency-domain coupled-mode models then combine these into fully vectorial approximations for the optical electromagnetic fields of the composite structure. Following a discretization of amplitude functions by 1D finite elements, pro- cedures from the realm of finite-element numerics are applied to establish systems of linear equations for the then- discrete modal amplitudes. Examples substantiate the functioning of the technique and allow for some numerical assessment. The full 3D simulations are highly efficient in memory consumption, moderately demanding in com- putational time, and, in regimes of low radiative losses, sufficiently accurate for practical design. Our results include the perturbation of guided modes by changes of the refractive indices, the interaction of waves in parallel, horizontally or vertically coupled straight waveguides, and a series of crossings of potentially overlapping channels with fairly arbitrary relative positions and orientations.

The modal properties of curved dielectric slab waveguides are investigated. We consider quasi-confined, attenuated modes that propagate at oblique angles with respect to the axis through the center of curvature. Our analytical model describes the transition from scalar 2-D TE/TM bend modes to lossless spiral waves at near-axis propagation angles, with a continuum of vectorial attenuated spiral modes in between. Modal solutions are characterized in terms of directional wavenumbers and attenuation constants. Examples for vectorial mode profiles illustrate the effects of oblique wave propagation along the curved slab segments. For the regime of lossless spiral waves, the relation with the guided modes of corresponding dielectric tubes is demonstrated.

Controlling light emission out of subwavelength nanoslit/aperture structures is of great important for highly integrated photonic circuits. Here we propose a new method to achieve direction-tunable emission based on a compact metallic microcavity with double nanoslit. Our method combines the principles of Young’s interference and surface plasmon polaritons interference. We show that the direction of the far-field beam can be controlled over a wide range of angles by manipulating the frequency and relative phase of light arriving at the two slits, which holds promise for applications in the ultracompact optoelectronic devices.

We successfully developed a process to fabricate freestanding cubic aluminium nitride (c-AlN) membranes containing cubic gallium nitride (c-GaN) quantum dots (QDs). The samples were grown by plasma assisted molecular beam epitaxy (MBE). To realize the photonic crystal (PhC) membrane we have chosen a triangular array of holes. The array was fabricated by electron beam lithography and several steps of reactive ion etching (RIE) with the help of a hard mask and an undercut of the active layer. The r/a- ratio of 0.35 was deter- mined by numerical simulations to obtain a preferably wide photonic band gap. Micro-photoluminescence (μ-PL) measurements of the photonic crystals, in particular of a H1 and a L3 cavity, and the emission of the QD ensemble were performed to characterize the samples. The PhCs show high quality factors of 4400 for the H1 cavity and about 5000/3000 for two different modes of the L3 cavity, respectively. The energy of the fundamental modes is in good agreement to the numerical simulations.

The problem of light scattering by ice crystals of cirrus clouds is considered in the case of a hexagonal ice plate with different distributions over crystal orientations. The physical-optics approximation based on (E, M)-diffraction theory is compared with two exact numerical methods: the finite difference time domain (FDTD) and the discontinuous Galerkin time domain (DGTD) in order to estimate its accuracy and limits of applicability. It is shown that the accuracy of the physical-optics approximation is estimated as 95% for the averaged backscattering Mueller matrix for particles with size parameter more than 120. Furthermore, the simple expression that allows one to estimate the minimal number of particle orientations required for appropriate spatial averaging has been derived.

We present phase sensitive cavity field measurements on photonic crystal microcavities. The experiments have been performed as autocorrelation measurements with ps double pulse laser excitation for resonant and detuned conditions. Measured E-field autocorrelation functions reveal a very strong detuning dependence of the phase shift between laser and cavity field and of the autocorrelation amplitude of the cavity field. The fully resolved phase information allows for a precise frequency discrimination and hence for a precise measurement of the detuning between laser and cavity. The behavior of the autocorrelation amplitude and phase and their detuning dependence can be fully described by an analytic model. Furthermore, coherent control of the cavity field is demonstrated by tailored laser excitation with phase and amplitude controlled pulses. The experimental proof and verification of the above described phenomena became possible by an electric detection scheme, which employs planar photonic crystal microcavity photo diodes with metallic Schottky contacts in the defect region of the resonator. The applied photo current detection was shown to work also efficiently at room temperature, which make electrically contacted microcavities attractive for real world applications.

e study the discrete soliton formation in one- and two- dimensional arrays of nanowires coated with graphene monolayers. Highly confined solitons, including the fundamental and the higher-order modes, are found to be supported by the proposed structure with a low level of power flow. Numerical analysis reveals that, by tuning the input intensity and Fermi energy, the beam diffraction, soliton dimension and propagation loss can be fully controlled in a broad range, indicating potential values of the graphene-based solitons in nonlinear/active nanophotonic systems.

We report on second harmonic generation spectroscopy on a series of rectangular arrays of split-ring resonators. Within the sample series, the lattice constants are varied, but the area of the unit cell is kept fixed. The SHG signal intensity of the different arrays upon resonant excitation of the fundamental plasmonic mode strongly depends on the respective arrangement of the split-ring resonators. This finding can be explained by variations of the electromagnetic interactions between the split-ring resonators in the different arrays. The experimental results are in agreement with numerical calculations based on the discontinuous Galerkin time-domain method. (PDF) The role of electromagnetic interactions.... Available from: https://www.researchgate.net/publication/297612326_The_role_of_electromagnetic_interactions_in_second_harmonic_generation_from_plasmonic_metamaterials [accessed Aug 13 2018].

We simulate light scattering by random irregular particles that have dimensions much larger than the wavelength of incident light at the size parameter of 𝑋=200 using the discontinuous Galerkin time domain method. A comparison of the DGTD solution for smoothly faceted particles with that obtained with a geometric optics model shows good agreement for the scattering angle curves of intensity and polarization. If a wavelength-scale surface roughness is introduced, diffuse scattering at rough interface results in smooth and featureless curves for all scattering matrix elements which is consistent with the laboratory measurements of real samples.

The physical optics approximations are derived from the Maxwell equations. The scattered field equations by Kirchhoff, Stratton-Chu, Kottler and Franz are compared and discussed. It is shown that in the case of faceted particles, these equations reduce to a sum of the diffraction integrals, where every diffraction integral is associated with one plane–parallel optical beam leaving a particle facet. In the far zone, these diffraction integrals correspond to the Fraunhofer diffraction patterns. The paper discusses the E-, M- and (E, M)-diffraction theories as applied to ice crystals of cirrus clouds. The comparison to the exact solution obtained by the discontinuous Galerkin time domain method shows that the Kirchhoff diffraction theory is preferable.

We study the formation of subwavelength solitons in binary metal-dielectric lattices. We show that the transverse modulation of the lattice constant breaks the fundamental plasmonic band and suppresses the discrete diffraction of surface plasmon waves. New types of plasmonic solitons are found, and their characteristics are analyzed. We also demonstrate the existence of photonic-plasmonic vector solitons and elucidate their propagation properties.

Sheets of slab waveguides with sharp corners are investigated. By means of rigorous numerical experiments, we look at oblique incidence of semi-guided plane waves. Radiation losses vanish beyond a certain critical angle of incidence. One can thus realize lossless propagation through 90-degree corner configurations, where the remaining guided waves are still subject to pronounced reflection and polarization conversion. A system of two corners can be viewed as a structure akin to a Fabry-Perot-interferometer. By adjusting the distance between the two partial reflectors, here the 90-degree corners, one identifies step-like configurations that transmit the semi-guided plane waves without radiation losses, and virtually without reflections. Simulations of semi-guided beams with in-plane wide Gaussian profiles show that the effect survives in a true 3-D framework.

Plasmon modes of the exact same individual gold nanoprisms are investigated through combined nanometer-resolved electron energy-loss spectroscopy (EELS) and cathodoluminescence (CL) measurements. We show that CL only probes the radiative modes, in contrast to EELS, which additionally reveals dark modes. The combination of both techniques on the same particles thus provides complementary information and also demonstrates that although the radiative modes give rise to very similar spatial distributions when probed by EELS or CL, their resonant energies appear to be different. We trace this phenomenon back to plasmon dissipation, which affects in different ways the plasmon signatures probed by these techniques. Our experiments are in agreement with electromagnetic numerical simulations and can be further interpreted within the framework of a quasistatic analytical model. We therefore demonstrate that CL and EELS are closely related to optical scattering and extinction, respectively, with the addition of nanometer spatial resolution.

The coherent state preparation and control of single quantum systems is an important prerequisite for the implementation of functional quantum devices. Prominent examples for such systems are semiconductor quantum dots, which exhibit a fine structure split single exciton state and a V-type three level structure, given by a common ground state and two distinguishable and separately excitable transitions. In this work we introduce a novel concept for the preparation of a robust inversion by the sequential excitation in a V-type system via distinguishable paths.

We show how to optically connect guiding layers at different elevations in a 3-D integrated photonic circuit. Transfer of optical power carried by planar, semi-guided waves is possible without reflections or radiation losses, and over large vertical distances. This functionality is realized through simple step-like folds of high-contrast dielectric slab waveguides, in combination with oblique wave incidence, and fulfilling a resonance condition. Radiation losses vanish, and polarization conversion is suppressed for TE wave incidence beyond certain critical angles. This can be understood by fundamental arguments resting on a version of Snell’s law. The two 90° corners of a step act as identical partial reflectors in a Fabry–Perot-like resonator setup. By selecting the step height, i.e., the distance between the reflectors, one realizes resonant states with full transmission. Rigorous quasi-analytical simulations for typical silicon/silica parameters demonstrate the functioning. Combinations of several step junctions can lead to other types of optical on-chip connects, e.g., U-turn- or bridge-like configurations.

Microresonators containing quantum dots find application in devices like single photon emitters for quantum information technology as well as low threshold laser devices. We demonstrate the fabrication of 60 nm thin zinc-blende AlN microdisks including cubic GaN quantum dots using dry chemical etching techniques. Scanning electron microscopy analysis reveals the morphology with smooth surfaces of the microdisks. Micro-photoluminescence measurements exhibit optically active quantum dots. Furthermore this is the first report of resonator modes in the emission spectrum of a cubic AlN microdisk.

Whispering gallery modes (WGMs) were observed in 60 nm thin cubic AlN microdisk resonators containing a single layer of non-polar cubic GaN quantum dots. Freestanding microdisks were patterned by means of electron beam lithography and a two step reactive ion etching process. Micro-photoluminescence spectroscopy investigations were performed for optical characterization. We analyzed the mode spacing for disk diameters ranging from 2-4 lm. Numerical investigations using three dimensional finite difference time domain calculations were in good agreement with the experimental data. Whispering gallery modes of the radial orders 1 and 2 were identified by means of simulated mode field distributions.

Using a finite-difference time-domain method, we theoretically investigate the optical spectra of crossing perpendicular photonic crystal waveguides with quantum dots embedded in the central rod. The waveguides are designed so that the light mainly propagates along one direction and the cross talk is greatly reduced in the transverse direction. It is shown that when a quantum dot (QD) is resonant with the cavity, strong coupling can be observed via both the transmission and crosstalk spectrum. If the cavity is far off-resonant from the QD, both the cavity mode and the QD signal can be detected in the transverse direction since the laser field is greatly suppressed in this direction. This structure could have strong implications for resonant excitation and in-plane detection of QD optical spectroscopy.

We study the quantum properties and statistics of photons emitted by a quantum-dot biexciton inside a cavity. In the biexciton-exciton cascade, fine-structure splitting between exciton levels degrades polarization-entanglement for the emitted pair of photons. However, here we show that the polarization-entanglement can be preserved in such a system through simultaneous emission of two degenerate photons into cavity modes tuned to half the biexciton energy. Based on detailed theoretical calculations for realistic quantum-dot and cavity parameters, we quantify the degree of achievable entanglement.

Optical experiments on second-harmonic generation from split-ring-resonator square arrays show a nonmonotonic dependence of the conversion efficiency on the lattice constant. This finding is interpreted in terms of a competition between dilution effects and linewidth or near-field changes due to interactions among the individual elements in the array.

We numerically investigate the interaction dynamics of coupled cavities in planar photonic crystal slabs in different configurations. The single cavity is optimized for a long lifetime of the fundamental mode, reaching a Q-factor of ≈43, 000 using the method of gentle confinement. For pairs of cavities we consider several configurations and present a setup with strongest coupling observable as a line splitting of about 30 nm. Based on this configuration, setups with three cavities are investigated.

We demonstrate by spin quantum beat spectroscopy that in undoped symmetric (110)-oriented GaAs/AlGaAs single quantum wells, even a symmetric spatial envelope wave function gives rise to an asymmetric in-plane electron Land´e g-factor. The anisotropy is neither a direct consequence of the asymmetric in-plane Dresselhaus splitting nor a direct consequence of the asymmetric Zeeman splitting of the hole bands, but rather it is a pure higher-order effect that exists as well for diamond-type lattices. The measurements for various well widths are very well described within 14 × 14 band k·p theory and illustrate that the electron spin is an excellent meter variable for mapping out the internal—otherwise hidden—symmetries in two-dimensional systems. Fourth-order perturbation theory yields an analytical expression for the strength of the g-factor anisotropy, providing a qualitative understanding of the observed effects.

We study the influence of the phonon environment on the electron dynamics in a doped quantum dot molecule. A non-perturbative quantumkinetic theory based on correlation expansion is used in order to describe both diagonal and off-diagonal electron-phonon couplings representing real and virtual processes with relevant acoustic phonons. We show that the relaxation is dominated by phononassisted electron tunneling between constituent quantum dots and occurs on a picosecond time scale. The dependence of the time evolution of the quantum dot occupation probabilities on the energy mismatch between the quantum dots is studied in detail.